Deselect the specific checkbox of the row of aura lightning dataTable

I am using aura lightning dataTable to show the records with the checkbox, when click on the checkbox the selected rows printing below the dataTable and now I want that, when remove any of the selected records then the same record checkbox of the dataTable should be deselect.

In the above screenshot if I will remove

In the above screenshot if remove AE User21 pills then it should deselect same name row checkbox.

<lightning:datatable
                    keyField="id"
                    columns="{!v.columnsCopy }"
                    data="{!v.data}"
                    hideCheckBoxColumn="true"
                    defaultSortDirection="{!v.defaultSortDirection}"
                    sortedDirection="{!v.sortDirection}"
                    sortedBy="{!v.sortedBy}"
                    onsort="{!c.handleSort}"
                    onrowselection="{!c.handleSelect}"                 >
                    </lightning:datatable>

handleSelect : function(component, event, helper) {
    
    var selectedRows = event.getParam('selectedRows'); 
    var setRows = [];
    for ( var i = 0; i < selectedRows.length; i++ ) {
        
        setRows.push(selectedRows[i]);

    }
    component.set("v.selectedUsers", setRows);
    
    console.log('selectedUsers '+JSON.stringify(component.get('v.selectedUsers')));
    
}

removeUser:function(component, event, helper){
    var eventDataSet = event.target.dataset.index;
    alert('eventDataSet ' + eventDataSet);
    var Users = component.get('v.selectedUsers');
    Users.splice(Number(eventDataSet),1);
    component.set("v.selectedUsers", Users);
}